Publication Date

9-26-2024

Journal

International Journal of Molecular Sciences

DOI

10.3390/ijms251910333

PMID

39408663

PMCID

PMC11476625

PubMedCentral® Posted Date

9-26-2024

PubMedCentral® Full Text Version

Post-print

Published Open-Access

yes

Keywords

Female, Humans, Pregnancy, Biomarkers, Metabolomics, Adult, Pregnancy, Ectopic, Case-Control Studies, Metabolome, Tandem Mass Spectrometry, Chromatography, Liquid, Prospective Studies, ectopic pregnancy, gynecology, metabolomics, molecular networking, untargeted, biomarker, metabolite

Abstract

Ectopic pregnancy (EP) is the leading cause of maternal morbidity and mortality in the first trimester. Using an untargeted metabolomic approach, we sought to identify putative plasma biomarkers using tandem liquid chromatography-mass spectrometry for the detection of tubal EP. This case-control study included the prospective recruitment of 50 tubal EP cases and 50 early intrauterine pregnancy controls. To avoid over-fitting, logistic regression models were developed in a randomly selected discovery group (30 cases vs. 30 controls) and validated in the test group (20 cases vs. 20 controls). In total, 585 mass spectral features were detected, of which 221 molecular features were significantly altered in EP plasma (

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